Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N....

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Coulomb excitation of 184,186,188 Hg Nick Bree & Andrew Petts Katholieke Universiteit Leuven & University of Liverpool P.A. Butler, J. Cederkäll, E. Clement, T.E. Cocolios, L. Fraile, T. Grahn, M. Guttormsen, K. Hadynska, R.-D. Herzberg, M. Huyse, D.G. Jenkins, R. Julin, S. Knapen, Th. Kroell, R. Krücken, A.C. Larsen, P. Marley, P.J. Napiorkowski, J. Pakarinen, N. Patronis, P.J. Peura, E. Piselli, M. Scheck, S. Siem, I. Stefanescu, J. Van de Walle, P. Van Duppen, D. Voulot, F. Wenander and M. Zielinska

Transcript of Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N....

Page 1: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulomb excitation of 184,186,188HgNick Bree & Andrew Petts

Katholieke Universiteit Leuven & University of LiverpoolP.A. Butler, J. Cederkäll, E. Clement, T.E. Cocolios, L. Fraile, T. Grahn, M. Guttormsen, K. Hadynska, R.-D.

Herzberg, M. Huyse, D.G. Jenkins, R. Julin, S. Knapen, Th. Kroell, R. Krücken, A.C. Larsen, P. Marley, P.J.

Napiorkowski, J. Pakarinen, N. Patronis, P.J. Peura, E. Piselli, M. Scheck, S. Siem, I. Stefanescu, J. Van de

Walle, P. Van Duppen, D. Voulot, F. Wenander and M. Zielinska

Page 2: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Content

• Motivation: shape coexistence• Experimental set-up• Shape measurements by Coulomb

excitation• Preliminary experimental results• Conclusion and outlook

Coulex of 184,186,188Hg: Content

Page 3: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Z = 82

Coulex of 184,186,188Hg: Motivation

π

82

2d5/21h11/2

2d3/23s1/2

1g7/2

1h9/2

Page 4: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Motivation

184HgN=104

0+

2+

4+

0+

2+4+

0

367

1089

375

534653

0+

2+

4+

0

405

1080

523621808

0+2+4+

0+

2+

4+

0+2+

4+

0

413

1005

824881

1208

186HgN=106

188HgN=108

MID SHELL

Page 5: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Motivation

π=80

82

2d5/21h11/2

2d3/23s1/2

1g7/2

1h9/2

ν=104

126

2f7/21i13/2

3p3/22f5/2

1h9/2

3p1/2

2g9/2

E*intruder(4p-6h)=4(εjπ-εj’π) - ΔEππpair + ΔEπνM – ΔEπνQ

K. Heyde et al, Nucl. Phys. A 466, 189 (1987)

4(εjπ-εj’π)

ΔEπνQ~NπNν

2(εjπ-εj’π)

ΔEπνQ~NπNν

ΔEpairing

ΔEpairing

g.s. g.s.

Hg,Pb Pt,Po,Rn,Ra

184Hg

Slightly oblate ground state bandProlate band SHAPE COEXISTENCE

Page 6: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Experimental set-up

θP

θD

184Hg projectile

120Sn target

bϑ P

ϑ D

Page 7: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Experimental set-up

Isotope Charge state

Intensity@Miniball

184Hg 43+ 1000 pps

186Hg 43+ 2.0 x 105 pps

188Hg 44+ 2.5 x 105 pps

All 3 isotopes were post-accelerated by REX to 2.85 MeV/u.

Page 8: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Miniball

• Doppler shift in the gamma energy!

Coulex of 184,186,188Hg: Experimental set-up

θP

EP

ED

CD-detector

184Hg 2,85 MeV/u target 120Sn

2.3 mg/cm2

Page 9: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Shape measurements

0+

2+

+ + σ⎛ ⎞→ ⎜ ⎟Ω⎝ ⎠CEdB(E2 : 0 2 )

d

The cross section for exciting 184Hg to its 2+ state does not only depend on its reduced transition probability B(E2: 0+ -> 2+), but also on the diagonal matrix element <2+||M(E2)||2+>.

B(E2) = 19500±4500 e2fm4

N. Rud et al, PRL 31, 1421, 1973+ life time measurements

Since the B(E2) value is known, the sign and magnitude of the quadrupole moment of the 2+ state can be measured by calculating the excitation cross section out of the intensity ofthe detected γ photo peak of the 2+->0+ transition.

184Hg120Sn

184Hg

Page 10: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Preliminary experimental results

In August 2007 a Coulomb excitation experiment was performed on the neutron deficient 184,186,188Hg isotopes.

non Doppler corrected γ spectrumDoppler corrected γ spectrum

0+

2+

4+

0

367

1089

375

534653

0+

2+4+

Page 11: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Preliminary experimental results

In August 2007 a Coulomb excitation experiment was performed on the neutron deficient 184,186,188Hg isotopes.

non Doppler corrected γ spectrumDoppler corrected γ spectrum

0+

2+

4+

0

367

1089

375

534653

0+

2+4+

Page 12: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Preliminary experimental results

In August 2007 a Coulomb excitation experiment was performed on the neutron deficient 184,186,188Hg isotopes.

Doppler corrected γ spectrum

0+

2+

4+

0

405

1080

523621808

0+2+

4+

403

Page 13: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Preliminary experimental results

In August 2007 a Coulomb excitation experiment was performed on the neutron deficient 184,186,188Hg isotopes.

Doppler corrected γ spectrum

0+

2+

4+

0+2+

4+

0

413

1005

824881

1208

Page 14: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Preliminary experimental results

Example: determination of the <2+||M(E2)||2+> matrix element in 186Hg.

0,8

1

1,2

1,4

1,6

1,8

2

-2 -1 0 1 2 3

<2+1||E2||2+

1> [eb]

<0+ g.

s.||E

2||2+ 1>

[eb]

PRELIMINARY186Hg on 107Ag1σ confidence levelno multiple Coulex

Page 15: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Preliminary experimental results

Example: determination of the <2+||M(E2)||2+> matrix element in 186Hg.

0,8

1

1,2

1,4

1,6

1,8

2

-2 -1 0 1 2 3

<2+1||E2||2+

1> [eb]

<0+ g.

s.||E

2||2+ 1>

[eb]

PRELIMINARY186Hg on 107Ag1σ confidence levelno multiple Coulex

Page 16: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Preliminary experimental results

Example: determination of the <2+||M(E2)||2+> matrix element in 186Hg.

0,8

1

1,2

1,4

1,6

1,8

2

-2 -1 0 1 2 3

<2+1||E2||2+

1> [eb]

<0+ g.

s.||E

2||2+ 1>

[eb]

PRELIMINARY186Hg on 107Ag1σ confidence levelno multiple Coulex

Page 17: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Preliminary experimental results

Example: determination of the <2+||M(E2)||2+> matrix element in 186Hg.

0,8

1

1,2

1,4

1,6

1,8

2

-2 -1 0 1 2 3

<2+1||E2||2+

1> [eb]

<0+ g.

s.||E

2||2+ 1>

[eb]

Lifetime measurementD. Proetel et al., Phys. Lett. 48B, 102 (1974)

Page 18: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Conclusion and outlook

Conclusions:

The heavy 184,186,188Hg were successfully produced and post-accelerated by REX-ISOLDE.

Apart from the first 2+ state, also other states have been populated.

The detected γ yields of the photo peaks can be used to extract:

• transitional matrix elements (B(E2) values)• diagonal matrix elements (quadrupole moments)

This is done by the program GOSIA by fitting the matrix elements to produce the obtained γ yields by a χ2

minimization. (T. Czosnyka et al, GOSIA2)

Page 19: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Conclusion and outlook

Outlook:

A proposal for a Coulomb excitation experiment on 180,182Hg at REX-ISOLDE has been accepted.

A proposal for lifetime measurements in 184,186,188Hg at Argonne National Laboratory has been submitted.

Other experiments aiming at studying this heavy mass region have been proposed (Ra and Rn).

Page 20: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 68Ni: Challenges and analysis improvements

π

82

2d5/21h11/2

2d3/23s1/2

1g7/2

1h9/2

ν

126

2f7/21i13/2

3p3/22f5/2

1h9/2

3p1/2

2g9/2

π

82

2d5/21h11/2

2d3/23s1/2

1g7/2

1h9/2

Page 21: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Me a

n S

quar

e C

harg

e ra

dii <

r2 >

• Influence of intruder states on the <r2> values in Pt and Hg isotopes• Evidence for a deviation of the <r2> values from the DM in Pb’s around 190-194Pb

0

500

1000

1500

2000

2500

3000

0+

2+

4+

6+

174 178 182 186 190 194Mass Number

E*[keV]

Hg (Z=80)

0p-2h

2p-4h

100 105 110 115 120 125 130

=0.1 fm2

Pb

Hg

Pt

N=104 N=126

Neutron Number

Pb 0+ & l.s.Pb 13/2+

Hg 0+ & l.s.Hg h.s.Pt g.s.Pt isomer

DM

0p-4h2p-6h

Mass Number

0+2+

4+

6+

8+

176 180 184 188 192 196

E*[keV] Pt (Z=78)

N=104

190Pb

oexistence and <r2> in the Lea

Page 22: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Motivation

π=80

82

2d5/21h11/2

2d3/23s1/2

1g7/2

1h9/2

ν=106

126

2f7/21i13/2

3p3/22f5/2

1h9/2

3p1/2

2g9/2

0+2+

4+186Hg

0+

2+

4+

0

405

1080

523621808

Page 23: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Motivation

π=80

82

2d5/21h11/2

2d3/23s1/2

1g7/2

1h9/2

ν=108

126

2f7/21i13/2

3p3/22f5/2

1h9/2

3p1/2

2g9/2

188Hg

0+

2+

4+

0+2+

4+

0

413

1005

824881

1208

Page 24: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Preliminary experimental results

In August 2007 a Coulomb excitation experiment was performed on the neutron deficient 184,186,188Hg isotopes.

Doppler corrected γ spectrum

0+

2+

4+

0+2+

4+

0

413

1005

824881

1208Q>0

Q=0

Q<0

Page 25: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Q>0

Q=0

Q<0

Coulex of 184,186,188Hg: Preliminary experimental results

Page 26: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Motivation

π=80

82

2d5/21h11/2

2d3/23s1/2

1g7/2

1h9/2

ν=104

126

2f7/21i13/2

3p3/22f5/2

1h9/2

3p1/2

2g9/2

184Hg

0+0

2+

4+

367

1089

6+1549

8+2057

shell model: π0p2h states

mean-field approximation:

slightly oblateJ.L.Wood et al, Phys, Rep., 215, 3&4 (1992)

Page 27: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

Coulex of 184,186,188Hg: Motivation

π=80

82

2d5/21h11/2

2d3/23s1/2

1g7/2

1h9/2

ν=104

126

2f7/21i13/2

3p3/22f5/2

1h9/2

3p1/2

2g9/2

184Hg

0+0

2+

4+

367

1089

6+1549

8+2057

shell model: π4p6h states

mean-field approximation:

stronger prolatedeformation

0+375

2+4+

534653

6+994

8+1412

10+1901

J.L.Wood et al, Phys, Rep., 215, 3&4 (1992)

Page 28: Coulomb excitation of 184,186,188Hgegp-workshop.in2p3.fr/docs/Talks-Vendredi/Bree N. Gammapool.pdf · Hg,Pb Pt,Po,Rn,Ra 184Hg Slightly oblate ground state band Prolate band SHAPE

0+

2+

4+

0

367

1089

375

534653

0+

2+

4+

<18E0+E2

100

100 100